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VALORIZATION OF BIOGAS THROUGH SIMULTANEOUS CO AND HS REMOVAL BY RENEWABLE AQUEOUS AMMONIA SOLUTION IN

《农业科学与工程前沿（英文）》 2023年 第10卷 第3期   页码 468-478 doi: 10.15302/J-FASE-2022473

摘要：

● Simultaneous H2S and CO2 removal from biogas is studied.

关键词： biomethane     biogas purification     CO2 removal     H2S removal     membrane absorption    

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Review on cryogenic technologies for CO removal from natural gas

Yujing BI, Yonglin JU

《能源前沿（英文）》 2022年 第16卷 第5期   页码 793-811 doi: 10.1007/s11708-022-0821-0

摘要： CO2 in natural gas (NG) is prone to condense directly from gas to solid or solidify from liquid to solid at low temperatures due to its high triple point and boiling temperature, which can cause a block of equipment. Meanwhile, CO2 will also affect the calorific value of NG. Based on the above reasons, CO2 must be removed during the NG liquefaction process. Compared with conventional methods, cryogenic technologies for CO2 removal from NG have attracted wide attention due to their non-polluting and low-cost advantages. Its integration with NG liquefaction can make rational use of the cold energy and realize the purification of NG and the production of by-product liquid CO2. In this paper, the phase behavior of the CH4-CO2 binary mixture is summarized, which provides a basis for the process design of cryogenic CO2 removal from NG. Then, the detailed techniques of design and optimization for cryogenic CO2 removal in recent years are summarized, including the gas-liquid phase change technique and the gas-solid phase change technique. Finally, several improvements for further development of the cryogenic CO2 removal process are proposed. The removal process in combination with the phase change and the traditional techniques with renewable energy will be the broad prospect for future development.

关键词： cryogenic CO2 removal     purification of natural gas (NG)     biogas upgrading     CH4-CO2 binary system    

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Dehydration of natural gas and biogas streams using solid desiccants: a review

Soheil Bahraminia, Mansoor Anbia, Esmat Koohsaryan

《化学科学与工程前沿（英文）》 2021年 第15卷 第5期   页码 1050-1074 doi: 10.1007/s11705-020-2025-7

摘要： Natural gas and biogas are two mixtures that consist of methane as their main component. These two gas mixtures are usually saturated with water vapor, which cause many problems, such as damaging the gas processing equipment by increasing the gas’s corrosion potential or clogging the pipelines due to gas hydrate formation. Thus, removing water vapor from these gas streams is mandatory. In this review paper, the main dehydration methods have been overviewed, and scrutiny of the adsorption dehydration has been carried out. Furthermore, the most important solid desiccants and their improvements have been reviewed.

关键词： natural gas     biogas     dehydration     adsorption     solid desiccant    

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Distribution of PCDD/Fs in a food waste anaerobic digestion process with biogas utilization

《环境科学与工程前沿（英文）》 2023年 第17卷 第11期 doi: 10.1007/s11783-023-1736-7

摘要：

● The PCDD/F distribution patterns of the FW-AD process were investigated.

关键词： Biological treatment     MSW classification     Mass balance     Solid digestate    

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大型养殖场沼气工程

潘文智

《中国工程科学》 2011年 第13卷 第2期   页码 40-43

摘要：

结合国内外大中型沼气工程情况，以德青源沼气工程为例，介绍了农村废弃物变废为宝的工艺流程，提供了农村能源解决方案，并结合我国沼气工程现有问题提出几点建议，以使大中型沼气工程走向规范化。

关键词： 沼气工程     德青源沼气工程     核心技术     展望与建议    

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Influence of HS and NH on biogas dry reforming using Ni catalyst: a study on single and synergetic effect

《环境科学与工程前沿（英文）》 2023年 第17卷 第3期 doi: 10.1007/s11783-023-1632-1

摘要：

● NH3 in biogas had a slight inhibitory effect on dry reforming.

关键词： Biogas     Dry reforming     Sulfur poisoning     Ammonia     Synergetic effect     Hydrogen    

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Techno-economic evaluation of a biogas-based oxidative coupling of methane process for ethylene production

Alberto T. Penteado, Mijin Kim, Hamid R. Godini, Erik Esche, Jens-Uwe Repke

《化学科学与工程前沿（英文）》 2018年 第12卷 第4期   页码 598-618 doi: 10.1007/s11705-018-1752-5

摘要：

This contribution is a preliminary techno-economic assessment of a biogas-based oxidative coupling of methane (OCM) process. Biogas is frequently utilized as a renewable energy source within small scale combined heat and power plants or as a natural gas substitute. The activation of methane also enables its utilization as a feedstock to produce chemicals. In this sense, the OCM process allows for the direct conversion of methane into ethylene, which is a major building block for the chemical and polymer industries. Biogas resulting from the anaerobic digestion of vinasse, a liquid effluent from bioethanol industry, is treated for contaminant removal and its methane content is converted into ethylene, which is then purified as the main product. The biogas cleaning process is assessed based on literature data, while an experimentally validated simulation model is used to assess the OCM process. A techno-economic evaluation is then performed through a Monte Carlo simulation, wherein uncertain parameters take random values between reasonable bounds. The net present value results positive in 74% of the cases, indicating that the project is profitable under a wide range of scenarios. Some performance improvement opportunities have been identified and highlighted to guide future studies in the topic.

关键词： biogas conversion     ethylene production     oxidative coupling of methane     feasibility study    

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Bioinspired and biomimetic membranes for water purification and chemical separation: A review

《环境科学与工程前沿（英文）》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1412-8

摘要：

•The history of biological and artificial water channels is reviewed.

关键词： Aquaporins     Artificial water channels     Biomimetic membranes     Chemical separation and water purification    

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Advanced purification and comprehensive utilization of yellow phosphorous off gas

Ping NING,Xiangyu WANG

《环境科学与工程前沿（英文）》 2015年 第9卷 第2期   页码 181-189 doi: 10.1007/s11783-014-0698-1

摘要： Yellow phosphorous is an important raw material in the chemical industry. However, during the production of yellow phosphorous, high concentrations of carbon monoxide and other impurities are released. Without appropriate purification and removal, this off gas has potential to cause severe pollution problems once released. Purified yellow phosphorous off gas can be beneficially reused as a raw material in chemical production for synthesis of high value-added chemical reagents. In this paper, the significance of purification and reutilization of yellow phosphorous off gas are explored. The principles, processes, and main characteristics of the technologies for purification and reuse of yellow phosphorus off gas (including technical measurements of impurity reduction, relevant engineering cases, and public acceptance of the technologies) are summarized. In view of the existing problems and scientific development requirements, this paper proposes several recommendations for green production based on the concept of recycle economics. We conclude that advanced purification and comprehensive reutilization can be an effective solution for heavy pollution resulting from yellow phosphorous off gassing.

关键词： yellow phosphorous off gas     purification     comprehensive utilization    

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Purification of

Y. LIU, M. PIETZSCH, J. ULRICH

《化学科学与工程前沿（英文）》 2013年 第7卷 第1期   页码 37-42 doi: 10.1007/s11705-013-1303-z

摘要： Here a case study of -asparaginase II out of a recombinant is presented. The target protein was obtained by simple cell disintegration and acetone precipitation. The -asparaginase II has been crystallized in three different forms in the following microbatch crystallization. The rod-shaped crystals (~400 μm edge length) were obtained at either 8°C or 22°C after 17 h by addition of PEG . The rectangular-shaped crystals were obtained after further recrystallization of the rod-shaped crystals. The rhombic-shaped crystals formed at 8°C after 12 days when cold ethanol was used instead of PEG . All crystallizations were performed in tris-acetate buffer (50 mmol·L , pH 5.1). By crystallization, the specific activity of -asparaginase II has increased 5-fold. The protein content and the purity of the crystals were evaluated by sodium dodecyl sulfate polyacrylamide gel electrophoresis (SDS-PAGE). The more concentrated -asparaginase II out of an extract mixture and the presence of only less minor proteins after crystallization demonstrates that crystallization is an effective and mild method to purify the target protein. The single crystal X-ray diffraction pattern reveals that the crystals are proteins and the X-ray powder diffraction (XRPD) pattern shows clearly that the crystals forming in PEG and ethanol have different crystal structures.

关键词： protein crystallization     L-asparaginase II     purification    

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A hybrid fuel cell for water purification and simultaneously electricity generation

《环境科学与工程前沿（英文）》 2023年 第17卷 第1期 doi: 10.1007/s11783-023-1611-6

摘要：

● A novel hybrid fuel cell (F-HFC) was fabricated.

关键词： Flow-through field     Hybrid fuel cell     Polyoxometalates     Water purification     Electricity generation    

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Techno-economic assessment of providing control energy reserves with a biogas plant

Ervin Saracevic, David Woess, Franz Theuretzbacher, Anton Friedl, Angela Miltner

《化学科学与工程前沿（英文）》 2018年 第12卷 第4期   页码 763-771 doi: 10.1007/s11705-018-1776-x

摘要：

Grid stability is being challenged by the increasing integration of power plants with volatile power generation into the energy system. Power supply fluctuations must be compensated by energy system flexibility. The storability of the energy carrier enables biogas plants to generate power flexibly. In this study, the technical and economic effects of providing positive secondary control energy reserves with an Austrian biogas plant were assessed. The plant’s main focus lies in biomethane production with the option of heat and power generation through combined heat and power (CHP) units. A detailed simulation model of the investigated biogas plant was developed, which is presented in this work. Ex-post simulations of one year of flexible plant operation were conducted with this model. The findings show that the installed biogas storage capacity is sufficient to provide control energy reserves while simultaneously producing biomethane. Profitability of providing control energy reserves largely depends on the prices at the control energy market and on CHP unit start-up costs. A cost efficiency analysis demonstrated that investing in a hot water tank with a volume of 5 m3 for short-term heat storage turned out to be economically viable.

关键词： biogas plant     process simulation     control energy reserves     economic assessment     gas storage    

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Biogas and its opportunities—A review

Panagiotis G. Kougias, Irini Angelidaki

《环境科学与工程前沿（英文）》 2018年 第12卷 第3期 doi: 10.1007/s11783-018-1037-8

摘要： Biogas production is a well-established technology primarily for the generation of renewable energy and also for the valorization of organic residues. Biogas is the end product of a biological mediated process, the so called anaerobic digestion, in which different microorganisms, follow diverse metabolic pathways to decompose the organic matter. The process has been known since ancient times and was widely applied at domestic households providing heat and power for hundreds of years. Nowadays, the biogas sector is rapidly growing and novel achievements create the foundation for constituting biogas plants as advanced bioenergy factories. In this context, the biogas plants are the basis of a circular economy concept targeting nutrients recycling, reduction of greenhouse gas emissions and biorefinery purposes. This review summarizes the current state-of-the-art and presents future perspectives related to the anaerobic digestion process for biogas production. Moreover, a historical retrospective of biogas sector from the early years of its development till its recent advancements gives an outlook of the opportunities that are opening up for process optimisation.

关键词： Anaerobic digestion     Biogas     Biowastes     Solid waste     Manure     Industrial waste    

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Pressure swing adsorption/membrane hybrid processes for hydrogen purification with a high recovery

Baojun Li,Gaohong He,Xiaobin Jiang,Yan Dai,Xuehua Ruan

《化学科学与工程前沿（英文）》 2016年 第10卷 第2期   页码 255-264 doi: 10.1007/s11705-016-1567-1

摘要： Hydrogen was recovered and purified from coal gasification-produced syngas using two kinds of hybrid processes: a pressure swing adsorption (PSA)-membrane system (a PSA unit followed by a membrane separation unit) and a membrane-PSA system (a membrane separation unit followed by a PSA unit). The PSA operational parameters were adjusted to control the product purity and the membrane operational parameters were adjusted to control the hydrogen recovery so that both a pure hydrogen product (>99.9%) and a high recovery (>90%) were obtained simultaneously. The hybrid hydrogen purification processes were simulated using HYSYS and the processes were evaluated in terms of hydrogen product purity and hydrogen recovery. For comparison, a PSA process and a membrane separation process were also used individually for hydrogen purification. Neither process alone produced high purity hydrogen with a high recovery. The PSA-membrane hybrid process produced hydrogen that was 99.98% pure with a recovery of 91.71%, whereas the membrane-PSA hybrid process produced hydrogen that was 99.99% pure with a recovery of 91.71%. The PSA-membrane hybrid process achieved higher total H recoveries than the membrane-PSA hybrid process under the same H recovery of membrane separation unit. Meanwhile, the membrane-PSA hybrid process achieved a higher total H recovery (97.06%) than PSA-membrane hybrid process (94.35%) at the same H concentration of PSA feed gas (62.57%).

关键词： hydrogen purification     PSA     membrane separation     hybrid process    

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Nanofiltration for separation and purification of saccharides from biomass

Xianhui Li, Sheng Tan, Jianquan Luo, Manuel Pinelo

《化学科学与工程前沿（英文）》 2021年 第15卷 第4期   页码 837-853 doi: 10.1007/s11705-020-2020-z

摘要： Saccharide production is critical to the development of biotechnology in the field of food and biofuel. The extraction of saccharide from biomass-based hydrolysate mixtures has become a trend due to low cost and abundant biomass reserves. Compared to conventional methods of fractionation and recovery of saccharides, nanofiltration (NF) has received considerable attention in recent decades because of its high selectivity and low energy consumption and environmental impact. In this review the advantages and challenges of NF based technology in the separation of saccharides are critically evaluated. Hybrid membrane processes, i.e., combining NF with ultrafiltration, can complement each other to provide an efficient approach for removal of unwanted solutes to obtain higher purity saccharides. However, use of NF membrane separation technology is limited due to irreversible membrane fouling that results in high capital and operating costs. Future development of NF membrane technology should therefore focus on improving material stability, antifouling ability and saccharide targeting selectivity, as well as on engineering aspects such as process optimisation and membrane module design.

关键词： saccharides     nanofiltration membrane     hybrid membrane process     biomas    

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标题 作者 时间 类型 操作

VALORIZATION OF BIOGAS THROUGH SIMULTANEOUS CO AND HS REMOVAL BY RENEWABLE AQUEOUS AMMONIA SOLUTION IN

期刊论文

Review on cryogenic technologies for CO removal from natural gas

Yujing BI, Yonglin JU

期刊论文

Dehydration of natural gas and biogas streams using solid desiccants: a review

Soheil Bahraminia, Mansoor Anbia, Esmat Koohsaryan

期刊论文

Distribution of PCDD/Fs in a food waste anaerobic digestion process with biogas utilization

期刊论文

大型养殖场沼气工程

潘文智

期刊论文

Influence of HS and NH on biogas dry reforming using Ni catalyst: a study on single and synergetic effect

期刊论文

Techno-economic evaluation of a biogas-based oxidative coupling of methane process for ethylene production

Alberto T. Penteado, Mijin Kim, Hamid R. Godini, Erik Esche, Jens-Uwe Repke

期刊论文

Bioinspired and biomimetic membranes for water purification and chemical separation: A review

期刊论文

Advanced purification and comprehensive utilization of yellow phosphorous off gas

Ping NING,Xiangyu WANG

期刊论文

Purification of

Y. LIU, M. PIETZSCH, J. ULRICH

期刊论文

A hybrid fuel cell for water purification and simultaneously electricity generation

期刊论文

Techno-economic assessment of providing control energy reserves with a biogas plant

Ervin Saracevic, David Woess, Franz Theuretzbacher, Anton Friedl, Angela Miltner

期刊论文

Biogas and its opportunities—A review

Panagiotis G. Kougias, Irini Angelidaki

期刊论文

Pressure swing adsorption/membrane hybrid processes for hydrogen purification with a high recovery

Baojun Li,Gaohong He,Xiaobin Jiang,Yan Dai,Xuehua Ruan

期刊论文

Nanofiltration for separation and purification of saccharides from biomass

Xianhui Li, Sheng Tan, Jianquan Luo, Manuel Pinelo

期刊论文